Rational design of catalysts for non-thermal plasma (NTP) catalysis: A reflective review

Shanshan Xu; Huanhao Chen; Xiaolei Fan

doi:10.1016/j.cattod.2023.114144

Rational design of catalysts for non-thermal plasma (NTP) catalysis: A reflective review

Shanshan Xu, Huanhao Chen, Xiaolei Fan

CBI Green Chemicals and Energy Centre

Research output: Journal Publication › Article › peer-review

19 Citations (Scopus)

Abstract

Non thermal plasma catalysis (NTP-catalysis) has shown the unique characteristics to enable many challenging chemical conversions under mild conditions. However, to date catalyst design with carefully consideration of the features of NTP activation was less achieved. In this reflective review, we revisited our previous research critically to comment on the rational and irrational aspects of these studies regarding catalyst design for selected NTP-catalytic systems, that is, CO₂ methanation, dry reforming of methane with CO₂, and NH₃ synthesis. Additionally, comments on catalyst design in relation to relevant literature on the NTP-catalytic systems above, especially CO₂ methanation, were also made. Based on that we devised relevant suggestion and prospect on rational design of bespoke catalysts for NTP-catalysis, which can be beneficial to advance NTP-catalysis technologies.

Original language	English
Article number	114144
Journal	Catalysis Today
Volume	419
DOIs	https://doi.org/10.1016/j.cattod.2023.114144
Publication status	Published - 1 Jul 2023

Keywords

CO methanation
Catalysis
Catalyst design
Dry reforming of methane (DRM)
NH synthesis
Non-thermal plasma (NTP)

ASJC Scopus subject areas

Catalysis
General Chemistry

UN SDGs

This output contributes to the following UN Sustainable Development Goals (SDGs)

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10.1016/j.cattod.2023.114144

Cite this

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abstract = "Non thermal plasma catalysis (NTP-catalysis) has shown the unique characteristics to enable many challenging chemical conversions under mild conditions. However, to date catalyst design with carefully consideration of the features of NTP activation was less achieved. In this reflective review, we revisited our previous research critically to comment on the rational and irrational aspects of these studies regarding catalyst design for selected NTP-catalytic systems, that is, CO2 methanation, dry reforming of methane with CO2, and NH3 synthesis. Additionally, comments on catalyst design in relation to relevant literature on the NTP-catalytic systems above, especially CO2 methanation, were also made. Based on that we devised relevant suggestion and prospect on rational design of bespoke catalysts for NTP-catalysis, which can be beneficial to advance NTP-catalysis technologies.",

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AU - Chen, Huanhao

AU - Fan, Xiaolei

PY - 2023/7/1

Y1 - 2023/7/1

N2 - Non thermal plasma catalysis (NTP-catalysis) has shown the unique characteristics to enable many challenging chemical conversions under mild conditions. However, to date catalyst design with carefully consideration of the features of NTP activation was less achieved. In this reflective review, we revisited our previous research critically to comment on the rational and irrational aspects of these studies regarding catalyst design for selected NTP-catalytic systems, that is, CO2 methanation, dry reforming of methane with CO2, and NH3 synthesis. Additionally, comments on catalyst design in relation to relevant literature on the NTP-catalytic systems above, especially CO2 methanation, were also made. Based on that we devised relevant suggestion and prospect on rational design of bespoke catalysts for NTP-catalysis, which can be beneficial to advance NTP-catalysis technologies.

AB - Non thermal plasma catalysis (NTP-catalysis) has shown the unique characteristics to enable many challenging chemical conversions under mild conditions. However, to date catalyst design with carefully consideration of the features of NTP activation was less achieved. In this reflective review, we revisited our previous research critically to comment on the rational and irrational aspects of these studies regarding catalyst design for selected NTP-catalytic systems, that is, CO2 methanation, dry reforming of methane with CO2, and NH3 synthesis. Additionally, comments on catalyst design in relation to relevant literature on the NTP-catalytic systems above, especially CO2 methanation, were also made. Based on that we devised relevant suggestion and prospect on rational design of bespoke catalysts for NTP-catalysis, which can be beneficial to advance NTP-catalysis technologies.

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KW - Catalysis

KW - Catalyst design

KW - Dry reforming of methane (DRM)

KW - NH synthesis

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Rational design of catalysts for non-thermal plasma (NTP) catalysis: A reflective review

Abstract

Keywords

ASJC Scopus subject areas

UN SDGs

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